The magnetic ordering in high magnetoresistance Mn-doped ZnO thin films
Author(s) -
S. Venkatesh,
Abdulaziz Baras,
J.-S. Lee,
Iman S. Roqan
Publication year - 2016
Publication title -
aip advances
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.421
H-Index - 58
ISSN - 2158-3226
DOI - 10.1063/1.4944954
Subject(s) - superparamagnetism , condensed matter physics , polaron , magnetoresistance , ferromagnetism , colossal magnetoresistance , variable range hopping , materials science , magnetic semiconductor , doping , metal–insulator transition , magnetization , giant magnetoresistance , metal , thermal conduction , electron , magnetic field , physics , quantum mechanics , metallurgy , composite material
We studied the nature of magnetic ordering in Mn-doped ZnO thin films that exhibited ferromagnetism at 300 K and superparamagnetism at 5 K. We directly inter-related the magnetisation and magnetoresistance by invoking the polaron percolation theory and variable range of hopping conduction below the metal-to-insulator transition. By obtaining a qualitative agreement between these two models, we attribute the ferromagnetism to the s-d exchange-induced spin splitting that was indicated by large positive magnetoresistance (∼40 %). Low temperature superparamagnetism was attributed to the localization of carriers and non-interacting polaron clusters. This analysis can assist in understanding the presence or absence of ferromagnetism in doped/un-doped ZnO
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