Enhanced photocatalytic H2 evolution over CdS/Au/g-C3N4 composite photocatalyst under visible-light irradiation
Author(s) -
Xiaoling Ding,
Yingxuan Li,
Jie Zhao,
Yunqing Zhu,
Yan Li,
Wenye Deng,
Chuanyi Wang
Publication year - 2015
Publication title -
apl materials
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.571
H-Index - 60
ISSN - 2166-532X
DOI - 10.1063/1.4926935
Subject(s) - photocatalysis , materials science , visible spectrum , heterojunction , irradiation , composite number , reagent , hydrogen production , photochemistry , chemical engineering , hydrogen , catalysis , optoelectronics , composite material , chemistry , biochemistry , physics , organic chemistry , nuclear physics , engineering
A novel heterojunction structured composite photocatalyst CdS/Au/g-C3N4 has been developed by depositing CdS/Au with a core (Au)-shell (CdS) structure on the surface of g-C3N4. The photocatalytic hydrogen production activity of the developed photocatalyst was evaluated under visible-light irradiation (λ > 420 nm) using methanol as a sacrificial reagent. As a result, its activity is about 125.8 times higher than that of g-C3N4 and is even much higher than that of Pt/g-C3N4. The enhancement in photocatalytic activity is attributed to efficient separation of the photoexcited charges due to the anisotropic junction in the CdS/Au/g-C3N4 system
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