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Antiferromagnetic interaction in coupled CdSe/ZnMnSe quantum dot structures
Author(s) -
Daniel Dagnelund,
Qianqian Ren,
I. A. Buyanova,
Akihiro Murayama,
Weimin Chen
Publication year - 2012
Publication title -
applied physics letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.182
H-Index - 442
eISSN - 1077-3118
pISSN - 0003-6951
DOI - 10.1063/1.4739852
Subject(s) - exciton , quantum dot , photoluminescence , antiferromagnetism , excitation , magnetic semiconductor , biexciton , condensed matter physics , spectroscopy , semiconductor , circular polarization , polarization (electrochemistry) , materials science , optoelectronics , chemistry , molecular physics , physics , magnetic field , quantum mechanics
Spin polarization of nonmagnetic CdSe quantum dots (QDs) coupled to adjacent ZnMnSe diluted magnetic semiconductor (DMS) is investigated by CW and time-resolved magneto-optical spectroscopy under tunable laser excitation. Efficient enhancement in the degree of σ− circular polarization of photoluminescence from the CdSe QDs is observed under optical excitation at the σ+-active exciton state of the DMS. The fact that the enhancement persists much longer than the exciton lifetime of the DMS rules out a role of the DMS excitons. A possible explanation is discussed in terms of antiferromagnetic coupling between the excitons in QDs and aligned Mn ions in DMS.

funding agencies|Swedish Research Council|621-2007-4568621-2011-42542008-6582|Swedish Foundation for International Cooperation in Research and Higher Education (STINT)||Japan Society for the Promotion of Science||

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