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Results of polarized Raman spectroscopy are reported and used to obtain complete assignment of the optical lattice modes of 1,2,4,5‐tetrabromobenzene crystals for both the beta and gamma phases. Similar information is provided for the beta phase of 1,2,4,5‐tetrachlorobenzene crystal. The results are compared with lattice‐dynamics calculations. Discrepancies with previously reported measurements and calculations are discussed and rationalized.

Assignment of the Raman active lattice vibrations in various phases of 1,2,4,5-tetrabromobenzene and 1,2,4,5-tetrachlorobenzene crystals