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Although in our earlier paper! we suggested that the synthesis of transition state theory and pseudodynamical Monte Carlo techniques would prove to be a singularly useful means of obtaining desorption rate data, it now appears clear that the inclusion of importance sampling makes this approach even more powerful. The method does, for example, overcome the usual problems associated with the simulation of intrinsically rare events, 6 while at the same time permitting the study of the adatom concentration effects which are practically inaccessible by other methods. It is, in fact, this rather unique versatility of the Monte Carlo-TST formalism which most strongly commends itself to those interested in investigating adsorption/desorption phenomena.

Erratum: Bispectral analysis as a probe of quasielastic light scattering intensity fluctuations [J. Chem. Phys. 7 2, 6123 (1980)]