Disentangling the Mn moments on different sublattices in the half-metallic ferrimagnet Mn3−xCoxGa
Author(s) -
Peter Klaer,
Catherine Jenkins,
Vajiheh Alijani,
J. Winterlik,
Benjamin Balke,
Claudia Felser,
H. J. Elmers
Publication year - 2011
Publication title -
applied physics letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.182
H-Index - 442
eISSN - 1077-3118
pISSN - 0003-6951
DOI - 10.1063/1.3592802
Subject(s) - ferrimagnetism , condensed matter physics , tetragonal crystal system , magnetization , magnetic moment , magnetic circular dichroism , spin polarization , fermi level , formula unit , chemistry , spin (aerodynamics) , metal , materials science , crystallography , physics , crystal structure , magnetic field , spectral line , quantum mechanics , electron , organic chemistry , thermodynamics
Ferrimagnetic Mn3-xCoxGa compounds have been investigated by magnetic circular dichroism in x-ray absorption (XMCD). Compounds with x>0.5 crystallize in the CuHg2Ti structure. A tetragonal distortion of the cubic structure occurs for x <= 0.5. For the cubic phase, magnetometry reveals a linearly increasing magnetization of 2x Bohr magnetons per formula unit obeying the generalized Slater-Pauling rule. XMCD confirms the ferrimagnetic character with Mn atoms occupying two different sublattices with antiparallel spin orientation and different degrees of spin localization and identifies the region 0.6
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