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Trilayer composites consisting of 0.9Pb(Zr0.52Ti0.48)O3–0.1Pb(Zn1/3Nb2/3)O3 (0.9 PZT-0.1 PZN) and Ni0.6Cu0.2Zn0.2Fe2O4 (NCZF) in the configuration NCZF-(0.9 PZT-0.1 PZN)-NCZF were synthesized using pressure assisted sintering. Composites with optimized magnetostrictive to piezoelectric thickness ratio showed a high magnetoelectric (ME) coefficient of 525 mV/cm Oe. Further enhancement in the magnitude of ME coefficient was obtained (595 mV/cm Oe) when the angle of applied dc magnetic field was changed to 45°. Changing the intermediate piezoelectric layer from single to trilayer stack geometry configuration leads to the realization of giant ME response of 782 mV/cm Oe in sintered composites.

Giant magnetoelectric effect in sintered multilayered composite structures