Optical observation of the 3sσgFΠu3 Rydberg state of N2 | Zendy

J. P. Sprengers | Zendy; E. Reinhold | Zendy; W. Ubachs | Zendy; K. G. H. Baldwin | Zendy; B. R. Lewis | Zendy

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Optical observation of the 3sσgFΠu3 Rydberg state of N2

Author(s) -

J. P. Sprengers,

E. Reinhold,

W. Ubachs,

K. G. H. Baldwin,

B. R. Lewis

Publication year - 2005

Publication title -

the journal of chemical physics

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.071

H-Index - 357

eISSN - 1089-7690

pISSN - 0021-9606

DOI - 10.1063/1.2062189

Subject(s) - rydberg formula , rydberg state , atomic physics , valence (chemistry) , ionization , spectroscopy , chemistry , resolution (logic) , rydberg atom , physics , ion , quantum mechanics , artificial intelligence , computer science , organic chemistry

Using ultrahigh-resolution 1 XUV+1 UV two-photon ionization laser spectroscopy, the F Πu3 ←X Σg+1 (0,0) transition of N2 has been optically observed for the first time, and the 3s σg F Πu3 (v=0) Rydberg level fully characterized with rotational resolution. The experimental spectroscopic parameters and predissociation level widths suggest strong interactions between the F state and the 3p π u G Πu3 Rydberg and C′ Πu3 valence states, analogous to those well known in the case of the isoconfigurational Πu1 states

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