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Transition to chemical turbulence
Author(s) -
Qi Ouyang,
Harry L. Swinney
Publication year - 1991
Publication title -
chaos an interdisciplinary journal of nonlinear science
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.971
H-Index - 113
eISSN - 1089-7682
pISSN - 1054-1500
DOI - 10.1063/1.165851
Subject(s) - turbulence , domain (mathematical analysis) , chemical reaction , physics , statistical physics , chemistry , mathematics , mechanics , mathematical analysis , biochemistry
Experiments have been conducted on Turing-type chemical spatial patterns and their variants in a quasi-two-dimensional open spatial reactor with a chlorite-iodide-malonic acid reaction. A variety of stationary spatial structures-hexagons, stripes, and mixed states-were observed, and transitions to these states were studied. For conditions beyond those corresponding to the emergence of patterns, a transition was observed from stationary spatial patterns to chemical turbulence, which is marked by a continuous motion of the pattern within a domain and of the grain boundaries between domains. The transition to chemical turbulence was analyzed by measuring the correlation length, the average pattern speed, and the total length of the domain boundaries. The emergence of chemical turbulence is accompanied by a large increase in the defects in the pattern, which suggests that this is an example of defect-mediated turbulence.

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