Selective formic acid dehydrogenation at low temperature over a RuO2/COF pre-catalyst synthesized on the gram scale | Zendy

Liliana P. L. Gonçalves | Zendy; David Benjamin Christensen | Zendy; Maria Meledina | Zendy; Laura M. Salonen | Zendy; Dmitri Y. Petrovykh | Zendy; Enrique CarbóArgibay | Zendy; Juliana P. S. Sousa | Zendy; O.S.G.P. Soares | Zendy; M.F.R. Pereira | Zendy; Søren Kegnæs | Zendy; Yury V. Kolen’ko | Zendy

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Selective formic acid dehydrogenation at low temperature over a RuO₂/COF pre-catalyst synthesized on the gram scale

Author(s) -

Liliana P. L. Gonçalves,

David Benjamin Christensen,

Maria Meledina,

Laura M. Salonen,

Dmitri Y. Petrovykh,

Enrique CarbóArgibay,

Juliana P. S. Sousa,

O.S.G.P. Soares,

M.F.R. Pereira,

Søren Kegnæs,

Yury V. Kolen’ko

Publication year - 2020

Publication title -

catalysis science and technology

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.635

H-Index - 115

eISSN - 2044-4761

pISSN - 2044-4753

DOI - 10.1039/d0cy00145g

Subject(s) - dehydrogenation , catalysis , formic acid , dispersion (optics) , metal , materials science , gram , inorganic chemistry , chemistry , chemical engineering , organic chemistry , physics , biology , bacteria , genetics , optics , engineering

A pre-catalyst, consisting of RuO2 nanoparticles and clusters anchored on TpBD-Me2 COF, was synthesized. During catalytic formic acid dehydrogenation, RuO2 undergoes in situ reduction to metallic Ru, forming an active and selective catalyst, which outperforms the commercial Ru–C catalyst. The chemical structure of the COF supporting material is maintained during stability testing.

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