Facet engineering in metal organic frameworks to improve their electrochemical activity for water oxidation | Zendy

Jiawei Wan | Zendy; Di Liu | Zendy; Hai Xiao | Zendy; Hongpan Rong | Zendy; Guan Sheng | Zendy; Feng Xie | Zendy; Dingsheng Wang | Zendy; Yadong Li | Zendy

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Facet engineering in metal organic frameworks to improve their electrochemical activity for water oxidation

Author(s) -

Jiawei Wan,

Di Liu,

Hai Xiao,

Hongpan Rong,

Guan Sheng,

Feng Xie,

Dingsheng Wang,

Yadong Li

Publication year - 2020

Publication title -

chemical communications

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.837

H-Index - 333

eISSN - 1364-548X

pISSN - 1359-7345

DOI - 10.1039/d0cc00700e

Subject(s) - facet (psychology) , electrochemistry , oxygen evolution , metal , materials science , nanotechnology , chemical engineering , computer science , chemistry , electrode , metallurgy , engineering , psychology , social psychology , personality , big five personality traits

The facet effect has been well demonstrated for nanocrystal catalysis, however it is rarely revealed in metal organic frameworks (MOFs). Herein, we present a facile way to construct 2D zeolitic imidazolate framework-67 (ZIF-67) with dominant exposure of the (002) facets. We discovered that the ZIF-67 (002) facet exhibited the highest catalytic activity for oxygen evolution reaction (OER) among the (002), (011), and (111) facets. Moreover, this facet engineering is also available for ZIF-8 nanocrystals.

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