Made-to-order porous electrodes for supercapacitors: MOFs embedded with redox-active centers as a case study | Zendy

Arijit Mallick | Zendy; Hanfeng Liang | Zendy; Osama Shekhah | Zendy; Jiangtao Jia | Zendy; Georges Mouchaham | Zendy; Aleksander Shkurenko | Zendy; Youssef Belmabkhout | Zendy; Husam N. Alshareef | Zendy; Mohamed Eddaoudi | Zendy

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Made-to-order porous electrodes for supercapacitors: MOFs embedded with redox-active centers as a case study

Author(s) -

Arijit Mallick,

Hanfeng Liang,

Osama Shekhah,

Jiangtao Jia,

Georges Mouchaham,

Aleksander Shkurenko,

Youssef Belmabkhout,

Husam N. Alshareef,

Mohamed Eddaoudi

Publication year - 2020

Publication title -

chemical communications

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.837

H-Index - 333

eISSN - 1364-548X

pISSN - 1359-7345

DOI - 10.1039/c9cc08860a

Subject(s) - supercapacitor , redox , porosity , electrode , order (exchange) , materials science , chemical engineering , nanotechnology , electrochemistry , chemistry , inorganic chemistry , business , composite material , engineering , finance

In this work, a pre-designed Zr-based-MOF encompassing an organic linker with a redox active core is synthesized and its structure-property relationship as a supercapacitor electrode is investigated. An enhanced performance is revealed by the combination of this MOF's high porosity and redox core incorporation, which alters its double-layer and pseudocapacitance, respectively. An increase in the capacitance performance by a factor of two is achieved via post-synthetic structure rigidification using organic pillars.

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