Improved transparency–nonlinearity trade-off with boroxine-based octupolar molecules | Zendy

Gilles Alcaraz | Zendy; Lisenn Euzénat | Zendy; Olivier Mongin | Zendy; Claudine Katan | Zendy; Isabelle Ledoux | Zendy; Joseph Zyss | Zendy; Mireille BlanchardDesce | Zendy; Michel Vaultier | Zendy

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Improved transparency–nonlinearity trade-off with boroxine-based octupolar molecules

Author(s) -

Gilles Alcaraz,

Lisenn Euzénat,

Olivier Mongin,

Claudine Katan,

Isabelle Ledoux,

Joseph Zyss,

Mireille BlanchardDesce,

Michel Vaultier

Publication year - 2003

Publication title -

chemical communications

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 1.837

H-Index - 333

eISSN - 1364-548X

pISSN - 1359-7345

DOI - 10.1039/b308664j

Subject(s) - transparency (behavior) , molecule , nonlinear system , harmonic , chemistry , nonlinear optics , scattering , chemical physics , materials science , molecular physics , optics , physics , quantum mechanics , organic chemistry , computer science , computer security

A series of octupolar molecules derived from the boroxine framework were designed and their optical nonlinearities were investigated by performing harmonic light scattering experiments in solution; the molecules were found to combine excellent transparency in the near UV-visible region (lambdamax < or = 280 nm) and significant first-order hyperpolarisabilities (up to beta(0) = 56 x 10(-30) esu).

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