
Revision of the stratospheric bomb 14 CO 2 inventory
Author(s) -
Hesshaimer Vago,
Levin Ingeborg
Publication year - 2000
Publication title -
journal of geophysical research: atmospheres
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 1.67
H-Index - 298
eISSN - 2156-2202
pISSN - 0148-0227
DOI - 10.1029/1999jd901134
Subject(s) - stratosphere , environmental science , atmosphere (unit) , meteorology , atmospheric sciences , nuclear weapon , climatology , physics , nuclear physics , geology
About 4900 values of 14 CO 2 activity have been measured on stratospheric air samples collected between 1953 and 1975 when the major nuclear weapon tests injected large amounts of 14 C into the atmosphere. However, the validity of these data published in Health and Safety Laboratory reports was repeatedly criticized and their relevance is thus usually denied in model studies tracing the global carbon cycle with bomb 14 CO 2 . To oppose this criticism, we perform here a comprehensive analysis of the measurements and calculate stratospheric bomb 14 CO 2 inventories for the period in question. We find out that the recognized weaknesses of the survey do not justify a general discrimination against the 14 CO 2 observations. Our 14 CO 2 inventories determined using numerical methods to interpolate the observations widely confirm the more “hand‐made” results from a former study by Telegadas [1971] except in the northern poleward stratosphere. We are also able to clear away the reasons commonly advanced to call into question the stratospheric bomb 14 CO 2 inventories by up to 20%. These findings rehabilitate the most extensive data set of stratospheric 14 CO 2 observations and establish them, together with our corresponding bomb 14 CO 2 inventories, as a valuable observational constraint which should be seriously accounted for in global carbon cycle models and in other studies relying on an accurate simulation of air mass transport in the atmosphere.