Plasmonic Control of Radiative Properties of Semiconductor Quantum Dots Coupled to Plasmonic Ring Cavities
Author(s) -
Aliaksandra Rakovich,
Pablo Albella,
Stefan A. Maier
Publication year - 2015
Publication title -
acs nano
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 5.554
H-Index - 382
eISSN - 1936-086X
pISSN - 1936-0851
DOI - 10.1021/nn506433e
Subject(s) - plasmon , quantum dot , radiative transfer , quantum , semiconductor , optoelectronics , ring (chemistry) , nanotechnology , field (mathematics) , physics , plasmonic nanoparticles , materials science , coupling (piping) , optics , quantum mechanics , chemistry , mathematics , organic chemistry , pure mathematics , metallurgy
In recent years, a lot of effort has been made to achieve controlled delivery of target particles to the hotspots of plasmonic nanoantennas, in order to probe and/or exploit the extremely large field enhancements produced by such structures. While in many cases such high fields are advantageous, there are instances where they should be avoided. In this work, we consider the implications of using the standard nanoantenna geometries when colloidal quantum dots are employed as target entities. We show that in this case, and for various reasons, dimer antennas are not the optimum choice. Plasmonic ring cavities are a better option despite low field enhancements, as they allow collective coupling of many quantum dots in a reproducible and predictable manner. In cases where larger field enhancements are required, or for larger quantum dots, nonconcentric ring-disk cavities can be employed instead.
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