Nanoscale Carrier Multiplication Mapping in a Si Diode
Author(s) -
Corentin Durand,
Pierre Capiod,
Maxime Berthe,
Jean-Philippe Nys,
Christophe Krzeminski,
Didier Stiévenard,
Christophe Delerue,
B. Grandidier
Publication year - 2014
Publication title -
nano letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 4.853
H-Index - 488
eISSN - 1530-6992
pISSN - 1530-6984
DOI - 10.1021/nl5022255
Subject(s) - scanning tunneling microscope , diode , materials science , silicon , quantum tunnelling , electron , optoelectronics , electron beam induced current , excited state , yield (engineering) , impact ionization , ionization , nanoscopic scale , diffusion , semiconductor , atomic physics , chemistry , nanotechnology , physics , ion , organic chemistry , quantum mechanics , metallurgy , thermodynamics
Carrier multiplication (CM), the creation of electron-hole pairs from an excited electron, has been investigated in a silicon p-n junction by multiple probe scanning tunneling microscopy. The technique enables an unambiguous determination of the quantum yield based on the direct measurement of both electron and hole currents that are generated by hot tunneling electrons. The combined effect of impact ionization, carrier diffusion, and recombination is directly visualized from the spatial mapping of the CM efficiency. Atomically well-ordered areas of the p-n junction surface sustain the highest CM rate, demonstrating the key role of the surface in reaching high yield.
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