Interface Control in Organic Electronics Using Mixed Monolayers of Carboranethiol Isomers | Zendy

Jaemyung Kim | Zendy; You Seung Rim | Zendy; Yongsheng Liu | Zendy; Andrew C. Serino | Zendy; John C. Thomas | Zendy; Huajun Chen | Zendy; Yang Yang | Zendy; Paul S. Weiss | Zendy

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Interface Control in Organic Electronics Using Mixed Monolayers of Carboranethiol Isomers

Author(s) -

Jaemyung Kim,

You Seung Rim,

Yongsheng Liu,

Andrew C. Serino,

John C. Thomas,

Huajun Chen,

Yang Yang,

Paul S. Weiss

Publication year - 2014

Publication title -

nano letters

Language(s) - English

Resource type - Journals

SCImago Journal Rank - 4.853

H-Index - 488

eISSN - 1530-6992

pISSN - 1530-6984

DOI - 10.1021/nl501081q

Subject(s) - monolayer , work function , dipole , molecular electronics , self assembled monolayer , nanotechnology , transistor , molecule , field effect transistor , materials science , electronics , fabrication , organic molecules , interface (matter) , chemistry , layer (electronics) , organic chemistry , electrical engineering , voltage , medicine , alternative medicine , gibbs isotherm , pathology , engineering

We employ mixed self-assembled monolayers of carboranethiols to alter the work function of gold and silver systematically. We use isomers of symmetric carboranethiol cage molecules to vary molecular dipole moments and directions, which enable work function tunability over a wide range with minimal alterations in surface energy. Mixed monolayers of carboranethiol isomers provide an ideal platform for the study and fabrication of solution-processed organic field-effect transistors; improved device performance is demonstrated by interface engineering.

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