Ultrafast Strong-Field Photoemission from Plasmonic Nanoparticles
Author(s) -
Péter Dombi,
Anton Hörl,
Péter Rácz,
István Márton,
Andreas Trügler,
Joachim R. Krenn,
Ulrich Hohenester
Publication year - 2013
Publication title -
nano letters
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 4.853
H-Index - 488
eISSN - 1530-6992
pISSN - 1530-6984
DOI - 10.1021/nl304365e
Subject(s) - plasmon , ultrashort pulse , electron , nanoscopic scale , nanoparticle , materials science , plasmonic nanoparticles , particle (ecology) , nanotechnology , field (mathematics) , chemical physics , optoelectronics , optics , physics , laser , oceanography , mathematics , quantum mechanics , geology , pure mathematics
We demonstrate the ultrafast generation of electrons from tailored metallic nanoparticles and unravel the role of plasmonic field enhancement in this process by comparing resonant and off-resonant particles, as well as different particle geometries. We find that electrons become strongly accelerated within the evanescent fields of the plasmonic nanoparticles and escape along straight trajectories with orientations governed by the particle geometry. These results establish plasmonic nanoparticles as versatile ultrafast, nanoscopic sources of electrons.
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