Polycyclic Aromatic Hydrocarbon Exposure in Household Air Pollution from Solid Fuel Combustion among the Female Population of Xuanwei and Fuyuan Counties, China
Author(s) -
George S. Downward,
Wei Hu,
Nat Rothman,
Boris Reiss,
Guoping Wu,
Fusheng Wei,
Robert S. Chapman,
Lützen Portengen,
Qing Lan,
Roel Vermeulen
Publication year - 2014
Publication title -
environmental science and technology
Language(s) - English
Resource type - Journals
eISSN - 1520-5851
pISSN - 0013-936X
DOI - 10.1021/es504102z
Subject(s) - stove , coal , polycyclic aromatic hydrocarbon , environmental science , environmental chemistry , coal combustion products , solid fuel , combustion , pollution , population , air pollution , particulates , waste management , environmental engineering , chemistry , environmental health , biology , engineering , medicine , ecology , organic chemistry
Exposure to polycyclic aromatic hydrocarbons (PAHs) from burning "smoky" (bituminous) coal has been implicated as a cause of the high lung cancer incidence in the counties of Xuanwei and Fuyuan, China. Little is known about variations in PAH exposure from throughout the region nor how fuel source and stove design affects exposure. Indoor and personal PAH exposure resulting from solid fuel combustion in Xuanwei and Fuyuan was investigated using repeated 24 h particle bound and gas-phase PAH measurements, which were collected from 163 female residents of Xuanwei and Fuyuan. 549 particle bound (283 indoor and 266 personal) and 193 gas phase (all personal) PAH measurements were collected. Mixed effect models indicated that PAH exposure was up to 6 times higher when burning smoky coal than smokeless coal and varied by up to a factor of 3 between different smoky coal geographic sources. PAH measurements from unventilated firepits were up to 5 times that of ventilated stoves. Exposure also varied between different room sizes and season of measurement. These findings indicate that PAH exposure is modulated by a variety of factors, including fuel type, coal source, and stove design. These findings may provide valuable insight into potential causes of lung cancer in the area.
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