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The electron-transport layer in planar perovskite solar cells plays an important role in improving photoelectric conversion efficiency. At present, the main electronic transmission materials in perovskite solar cells include TiO 2 , ZnO, WO 3 , ZrO 2 , SnO 2 , ZnO 2 , etc. This work mainly studies the electron-transport characteristics of six different electron-transport layers in perovskite solar cells. Based on the density functional theory, the electron-transport model of a solar cell doped with formamidinium iodide lead compound perovskite under six different electron-transport materials was constructed, and their effective electron mass and the mobility of carriers were obtained by optimizing the structure and theoretical calculation. The results show that the mobility of electrons in TiO 2 crystal is slightly higher than that of FA 0.75 Cs 0.25 Sn 0.5 Pb 0.5 I 3 carriers. Because of their high matching degree, it can be reasonably explained that titanium dioxide has been widely used in perovskite solar cells and achieved higher photoelectric conversion efficiency. In addition, the mobility of carriers in WO 3 and SnO 2 crystals is also high, so they also have great advantages in carrier transport. Due to its abundant, nontoxic, and low-pollution content, TiO 2 has become the most widely used electronic transmission layer material for solar cells. Furthermore, we have explored eight new semiconductor materials that have not yet been used in perovskite solar cells as the electron-transport layer. The calculation results show that Ta 2 O 5 and Bi 2 O 3 are promising materials for the electron-transport layer. This study provides a theoretical basis for seeking better electronic transmission materials for solar cells in the future.

Study on the Property of Electron-Transport Layer in the Doped Formamidinium Lead Iodide Perovskite Based on DFT