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Study on Denitration Performance of Solid Waste Blast Furnace Slag Catalysts under Different Preparation Processes
Author(s) -
Lu Zhao,
Lei Zhang,
Shu Hao,
Jia Yang,
Fang Bai,
Xiaosheng Chen
Publication year - 2020
Publication title -
acs omega
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.779
H-Index - 40
ISSN - 2470-1343
DOI - 10.1021/acsomega.0c03672
Subject(s) - bentonite , materials science , catalysis , decomposition , mixing (physics) , ground granulated blast furnace slag , chemical engineering , slag (welding) , municipal solid waste , molding (decorative) , hydrothermal circulation , yield (engineering) , waste management , metallurgy , chemistry , composite material , organic chemistry , cement , physics , quantum mechanics , engineering
In this article, blast furnace slag, a high-yield industrial solid waste, was taken as the research object and it was used as the main material. Bentonite was used as the binder, and water was added to shape the blast furnace slag into a small column. The denitration catalyst was prepared using different methods, its denitration performances were compared and analyzed, and the best preparation method and process parameters were screened. Results showed that bentonite will clearly improve denitration performance, and 4:1 blast furnace slag and bentonite was selected as the molding ratio to reduce the effect of bentonite on its performance, combined with the hardness and surface adhesion of the prepared carrier. Separately, the catalysts were prepared using citric acid impregnation, hydrothermal decomposition, and mixing method, and active Mn was loaded. Among them, the hydrothermal decomposition method cannot completely decompose in a closed kettle, resulting in a lower denitration performance. The catalyst prepared using the mixing method is superior to that prepared using the impregnation method because the active component prepared by the former was more uniformly dispersed, and simple and easy to operate, which can meet the needs of the excess denitration catalysts of small enterprises.

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