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Easily accessible green-light activatable (&gt;500 nm) photocages based on red-shifted, π-extended coumarin scaffolds are developed with uncaging efficiencies similar to those of recently introduced BODIPY derivatives. The photocages possess increased aqueous solubility, high absorption coefficients within the 450-600 nm range, and exceptionally high two-photon cross sections.

Green-Light Activatable, Water-Soluble Red-Shifted Coumarin Photocages