Adsorption Materials and Processes for Carbon Capture from Gas-Fired Power Plants: AMPGas
Author(s) -
J. A. A. Gibson,
Enzo Mangano,
Elenica Shiko,
Alex Greenaway,
Andrei V. Gromov,
Magdalena M. Łozińska,
Daniel Friedrich,
E. E. B. Campbell,
Paul A. Wright,
Stefano Brandani
Publication year - 2016
Publication title -
industrial and engineering chemistry research
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 0.878
H-Index - 221
eISSN - 1520-5045
pISSN - 0888-5885
DOI - 10.1021/acs.iecr.5b05015
Subject(s) - flue gas , adsorption , physisorption , amine gas treating , chemisorption , activated carbon , process engineering , gas separation , chemical engineering , chemistry , acid gas , separation process , materials science , organic chemistry , inorganic chemistry , chromatography , biochemistry , membrane , engineering
The key challenge in postcombustion capture from gas-fired power plants is related to the low CO2 concentration in the flue gas (4–8% by volume). This means that conventional amine processes will result in a relatively high energy penalty, whereas novel adsorbents and adsorption processes have the potential to improve the efficiency of separation. High-selectivity adsorbents are required to achieve relatively high CO2 uptake at low partial pressures, which means that the separation process should be based on either very strong physisorption or chemisorption with thermal regeneration. From the process point of view, the main challenge is to develop efficient separation processes with rapid thermal cycles. In this report we present a detailed overview of the methodology behind the development of novel materials and processes as part of the “Adsorption Materials and Processes for Gas-fired power plants” (AMPGas) project. Examples from a wide variety of materials tested are presented, and the design of an inn...
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