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High-Resolution Tritium Profile in an Ice Core from Camp Century, Greenland
Author(s) -
Jixin Qiao,
William Colgan,
Gunnar Jakobs,
S.P. Nielsen
Publication year - 2021
Publication title -
environmental science and technology
Language(s) - English
Resource type - Journals
SCImago Journal Rank - 2.851
H-Index - 397
eISSN - 1520-5851
pISSN - 0013-936X
DOI - 10.1021/acs.est.1c01975
Subject(s) - ice core , environmental science , northern hemisphere , arctic , climatology , explosive material , atmospheric sciences , nuclear weapon , physical geography , geology , oceanography , geography , physics , nuclear physics , archaeology
We measure 3 H in an ice core from Camp Century. The temporal distribution of 3 H concentration in the ice core corresponds generally well with the historical record of explosive yields of atmospheric nuclear weapons tests. Maximum 3 H values observed in 1962-1963 are comparable to those in ice core or precipitation in many other locations in the Northern Hemisphere. There is no indication that significan 3 H contamination was locally released into the air during the operation of the Camp Century reactor. It is, however, somewhat surprising that several prominen 3 H peaks are still observed after 1980. We suggest that these are associated with airborne 3 H releases from the civil nuclear industry. A wavelet analysis during 1970-2017 indicates the primary frequency of variability in the 3 H record is annual 3 H peaks. These annual peaks can be combined with the 3 H spikes from global fallout of known nuclear weapons tests to benchmark and evaluate theoretical ice core dating scales back to the 1950s. A positive correlation is observed between annual 3 H average concentration and variability of Arctic Oscillation (AO). This highlights the value of 3 H as a potential tracer for air masses and airborne pollutants in the Arctic.

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