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Diamond lattice magnets, formed by a framework of corner-sharing tetrahedraof magnetic cations, offer unique opportunities to realize novel states ofmatter for potential utility in information technology. However, research hasmostly focused on AB2X4 spinels with Td magnetic ions. This hinders theatomically enabled tunability of competing interactions at different energyscales and the ability to harness many-body electronic states in quantummaterials, making the discovery of quantum fluctuations and spin dynamics lessaccessible. We discover a new material CaCo2TeO6 featuring a diamond lattice oftwo distinct Oh-Co2+ sites. This material displays strong quantum fluctuations,increased competing magnetic exchange interactions, and field-inducedtunability of magnetic structures. The results demonstrate how simple,fundamental refinements in ligand fields can profoundly influence the phasespace of quantum matter.

Jeff = 1/2 Diamond Magnet CaCo2TeO6: A Pathway toward New Spin Physics and Quantum Functions