Magnetic ordering and structural distortion in a PrFeAsO single crystal studied by neutron and x-ray scattering
Physical Review. B./physical Review. BPeer ReviewedM. G. Kim +72021Journals
We report the magnetic ordering and structural distortion in PrFeAsO crystals, the basis compound for one of the oxypnictide superconductors, using high-resolution x-ray diffraction, neutron diffraction, and x-ray resonant magnetic scattering (XRMS). We find the structural tetragonal-to-orthorhombic phase transition at T S = 147 K , the AFM phase transition of the Fe moments at T Fe = 72 K , and the Pr AFM phase transition at T Pr = 21 K . Combined high-resolution neutron diffraction and XRMS show unambiguously that the Pr moments point parallel to the longer orthorhombic a axis and order antiferromagnetically along the a axis but ferromagnetically along the b and c directions in the stripelike AFM order. The temperature-dependent magnetic order parameter of the Pr moments shows no evidence for a reorientation of moments.
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