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The magnetic ground state of BaFe 12 O 19  (BFO) is investigated using X‐ray absorption spectra (XAS), X‐ray magnetic circular dichroism (XMCD), and neutron diffraction studies at 1.2 and 1.5 K, respectively. The XMCD measurements on single‐crystals of BFO in grazing‐incidence geometry reveal canting of the spins away from the  c ‐axis of the hexagonal unit cell. Single‐crystal neutron diffraction studies reveal magnetic satellite peaks along the  00l  reciprocal lattice row around the forbidden  l =  2 n  ± 1 positions confirming the conical‐type magnetic structure in the ground state of BFO. The observation of the conical magnetic structure of BFO opens the possibility of type‐II multiferroicity in undoped BFO.

physica status solidi (rrl) – rapid research letters

Evidence for Conical Magnetic Structure in M‐Type BaFe 12 O 19  Hexaferrite: A Combined Single‐Crystal X‐ray Magnetic Circular Dichroism and Neutron Diffraction Study