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Take a breath : An oxygen‐tolerant hydrogenase can be employed with a dye in a photocatalytic scheme for the generation of H 2 . The homogeneous system does not require a redox mediator and visible‐light irradiation yields high amounts of H 2  even in the presence of air.

Photocatalytic Hydrogen Evolution with a Hydrogenase in a Mediator‐Free System under High Levels of Oxygen