Coupling of Carbon Monoxide with Nitrogen Monoxide at a Frustrated Lewis Pair Template | Zendy

Ye KeYin | Zendy; Kehr Gerald | Zendy; Daniliuc Constantin G. | Zendy; Liu Lei | Zendy; Grimme Stefan | Zendy; Erker Gerhard | Zendy

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Coupling of Carbon Monoxide with Nitrogen Monoxide at a Frustrated Lewis Pair Template

Author(s) -

Ye KeYin,

Kehr Gerald,

Daniliuc Constantin G.,

Liu Lei,

Grimme Stefan,

Erker Gerhard

Publication year - 2016

Publication title -

angewandte chemie

Language(s) - English

Resource type - Journals

eISSN - 1521-3757

pISSN - 0044-8249

DOI - 10.1002/ange.201603760

Subject(s) - carbon monoxide , chemistry , frustrated lewis pair , coupling (piping) , lewis acids and bases , nitrogen , monoxide , carbon monoxide dehydrogenase , photochemistry , catalysis , inorganic chemistry , organic chemistry , materials science , metallurgy

Coupling of carbon monoxide with nitrogen monoxide was achieved at a frustrated Lewis pair template. This unique reaction uses hydride as an auxiliary, which reductively activates carbon monoxide at the frustrated Lewis pair. The CO/NO coupling reaction then takes place through a pathway involving a radical reaction in which the hydrogen atom auxiliary is eventually removed again.

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