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The effect of quantum confinement in the optical absorption spectra  of atomically thin α‐In 2 Se 3  crystals is studied, observing a huge thickness‐dependent shift in the optical band gap of exfoliated α‐In 2 Se 3  flakes. The band gap variation reported here is among the largest found in semiconductor crystals and spans a region of the near‐UV spectrum uncovered by other 2D semiconductors.

Strong Quantum Confinement Effect in the Optical Properties of Ultrathin α‐In 2 Se 3