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Liquid‐phase exfoliated few‐layer graphene flakes  are noncovalently functionalized with tailor‐made cationic water‐soluble perylene diimides. By using a straightforward dip‐coating approach, homogeneous ultrathin films consisting of interpenetrated nanoarchitectures can be achieved by incorporation of anionic ZnO nanoparticles. These 0D/2D assemblies pave the way for the development of novel graphene‐based composite materials.

Highly Integrated Organic–Inorganic Hybrid Architectures by Noncovalent Exfoliation of Graphite and Assembly with Zinc Oxide Nanoparticles