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The anisotropic thermal‐conductivity tensor of bulk black phosphorus  (BP) for 80 ≤ T  ≤ 300 K is reported. Despite the anisotropy, phonons are predominantly scattered by Umklapp processes in all the crystallographic orientations. It is also found that the phonon mean‐free‐paths of BP are rather long (up to 1 µm) in the through‐plane direction.

Temperature Dependence of Anisotropic Thermal‐Conductivity Tensor of Bulk Black Phosphorus