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An organic–inorganic halide CH 3 NH 3 SnI 3  perovskite  with significantly improved structural stability is obtained via pressure‐induced amorphization and recrystallization. In situ high‐pressure resistance measurements reveal an increased electrical conductivity by 300% in the pressure‐treated perovskite. Photocurrent measurements also reveal a substantial enhancement in visible‐light responsiveness. The mechanism underlying the enhanced properties is shown to be associated with the pressure‐induced structural modification.

Enhanced Structural Stability and Photo Responsiveness of CH 3 NH 3 SnI 3 Perovskite via Pressure‐Induced Amorphization and Recrystallization