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Anodic self‐organized TiO 2  nanostumps  are formed and exploited for self‐ordering dewetting of Au–Ag sputtered films. This forms ordered particle configurations at the tube top (crown position) or bottom (ground position). By dealloying from a minimal amount of noble metal, porous Au nanoparticles are then formed, which, when in the crown position, allow for a drastically improved photocatalytic H 2  production compared with nanoparticles produced by conventional dewetting processes.

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Efficient Photocatalytic H 2  Evolution: Controlled Dewetting–Dealloying to Fabricate Site‐Selective High‐Activity Nanoporous Au Particles on Highly Ordered TiO 2  Nanotube Arrays