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Non‐destructive chemical functionalization of graphene  for applications in electronic devices (e.g., sensors or transducers) is achieved via assembly of carbon nanomembrane (CNM)/single‐layer graphene (SLG) van der Waals heterostructures. The CNMs are 1 nm‐thick, dielectric molecular sheets terminated with functional amino groups. The structure and performance of heterostructured field‐effect transistors (FETs) are characterized by photoelectron/Raman spectroscopy and by electric transport measurements in vacuum, ambient conditions and water.

All‐Carbon Vertical van der Waals Heterostructures: Non‐destructive Functionalization of Graphene for Electronic Applications