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Organometallic hexahapto (η 6 )‐chromium metal complexation of single‐layer graphene , which involves constructive rehybridization of the graphene π‐system with the vacant chromium d π  orbital, leads to field effect devices which retain a high degree of the mobility with enhanced on‐off ratio. This η 6  mode of bonding is quite distinct from the modification in electronic structure induced by conventional covalent σ‐bond formation with creation of sp 3  carbon centers in graphene lattice and this chemistry is reversible.

Organometallic Hexahapto Functionalization of Single Layer Graphene as a Route to High Mobility Graphene Devices