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Experimental evidence of a nonvolatile electric‐pulse‐induced insulator‐to‐metal transition  and possible superconductivity in the Mott insulator GaTa 4 Se 8  is reported. Scanning tunneling microscopy experiments show that this unconventional response of the system to short electric pulses arises from a nanometer‐scale electronic phase separation generated in the bulk material (see figure).

Electric‐Pulse‐driven Electronic Phase Separation, Insulator–Metal Transition, and Possible Superconductivity in a Mott Insulator