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Self‐assembly is one of the crucial mechanisms allowing the design multifunctional materials. Soft hybrid materials contain components of different natures and exhibit competitive interactions which drive self‐organization into structures of a particular function. Here a novel type of a magnetic hybrid material where the molecular tilt can be manipulated through a delicate balance between the topologically‐assisted colloidal self‐assembly of magnetic nanoparticles and the anisotropic molecular interactions in a liquid crystal matrix is demonstrated.

Magnetic Tilting in Nematic Liquid Crystals Driven by Self‐Assembly