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Recently, two-dimensional (2D) bilayer magnetic systems have been widelystudied. Their interlayer magnetic interactions play a vital role in themagnetic properties. In this paper, we theoretically studied the interlayermagnetic interactions, magnetic states and ferroelectricity of $\pi$/3-twistedCrX$_2$ (X = Se, Te) bilayers ($\pi$/3-CrX$_2$). Our study reveals that thelateral shift could switch the magnetic state of the $\pi$/3-CrSe$_2$ betweeninterlayer ferromagnetic and antiferromagnetic, while just tuning the strengthof the interlayer antiferromagnetic interactions in $\pi$/3-CrTe$_2$.Furthermore, the lateral shift can alter the off-plane electric polarization inboth $\pi$/3-CrSe$_2$ and $\pi$/3-CrTe$_2$. These results show that stacking isan effective way to tune both the magnetic and ferroelectric properties of1T-CrX$_2$ bilayers, making the 1T-CrX$_2$ bilayers hold promise for 2Dspintronic devices.

Interlayer magnetic interactions and ferroelectricity in $\pi$/3-twisted CrX$_2$ (X = Se, Te) bilayers