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Organic semiconductors (OSCs) are suitable materials for spintronicsapplications as they form a spinterface when placed next to a ferromagnet,which in turn leads to novel functionalities. The evolution of spinterface cantune the global magnetic anisotropy, magnetization reversal, magnetizationdynamics, etc. Planar tris-(8-hydroxyquinoline)aluminum (Alq3) OSC has showntremendous potential for spintronics applications, thanks to its efficientspin-polarized current transport ability. Here, we establish the spinterfacewhen the Alq3 molecules are deposited on amorphous ferromagnetCo20Fe60B20(CFB). The $\pi$-d hybridization in CFB/Alq3 enhances the coercivefield and significantly modifies the shape and size of the magnetic domains. A$\sim$100% increase in uniaxial anisotropic energies and a reduction inmagnetic damping are also evident owing to the strong interfacialhybridization.

Spinterface Mediated Magnetic Properties of Co20Fe60B20/Alq3 Heterostructures