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Macroscopic-scale nanostructures, situated at the interface of nanostructuresand bulk materials, hold significant promise in the realm of thermoelectricmaterials. Nanostructuring presents a compelling avenue for enhancing materialthermoelectric performance as well as unlocking intriguing nanoscale phenomena,including spin-dependent thermoelectric effects. This is achieved whilepreserving high power output capabilities and ease of measurements related tothe overall macroscopic dimensions. Within this framework, the recentlydeveloped three-dimensional interconnected nanowire and nanotube networks,integrated into a flexible polymer membrane, emerge as promising candidates formacroscopic nanostructures. The flexibility of these composites also paves theway for advances in the burgeoning field of flexible thermoelectrics. In thisstudy, we demonstrate that the three-dimensional nanowire networks made offerromagnetic metals maintain the intrinsic bulk thermoelectric power of theirbulk constituent even for a diameter reduced to approximately 23 nm.Furthermore, we showcase the pioneering magneto-thermoelectric measurements ofthree-dimensional interconnected nickel nanotube networks. These macroscopicmaterials, comprising interconnected nanotubes, enable the development oflarge-area devices that exhibit efficient thermoelectric performance, whiletheir nanoscale tubular structures provide distinctive magneto-transportproperties. This research represents a significant step toward harnessing thepotential of macroscopic nanostructured materials in the field ofthermoelectrics.

Thermoelectric and magneto-transport characteristics of interconnected networks of ferromagnetic nanowires and nanotubes