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Rare-earth-based triangular-lattice magnets provide the fertile ground toexplore the exotic quantum magnetic state. Herein, we report a new family ofRE-based triangular-lattice magnets Ba6RE2Ti4O17(RE= rare earth ions)crystallized into the hexagonal structure with space group of P63 mmc, wheremagnetic rare earth ions form an ideal triangular lattice within the ab-planeand stack in an AA -type fashion along the c-axis. The low-temperature magneticsusceptibility results reveal all the serial compounds have the dominantantiferromagnetic interactions and an absence of magnetic ordering down to 1.8K. The magnetization and electron spin resonance results indicate distinctmagnetic anisotropy for the compounds with different RE ions. Moreover,Ba6Nd2Ti4O17 single crystal is successfully grown and it exhibits strong Isinglike anisotropy with magnetic easy-axis perpendicular to the triangle-latticeplane, being a candidate to explore quantum spin liquid state with dominantIsing-type interaction.

Ba6RE2Ti4O17 (RE= Nd, Sm,Gd, Dy-Yb): A family of quasi-two-dimensional triangular lattice magnets