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The Reiss theory for binary homogeneous nucleation in binary gas mixtures iscritically analysed and further developed. Based on the analysis of phase spacetrajectories in the supercritical zone of the phase transition, carried outwithin the framework of the theory of two-dimensional dynamical systems andsupplemented by the flux matching condition at the boundary of the criticalzone, it is shown how the theory should be modified. The proposed modificationis equivalent to the earlier modifications by Langer and Stauffer, based onadditional trial assumptions (ansatz) for solving the steady state equation forthe non-equilibrium size distribution function, but reveals and substantiatesthe approximation underlying their approach. The extension of the Reiss theoryto binary vapours in inert carrier (atmospheric) gases is justified.

Development of the Reiss theory for binary homogeneous nucleation of aerosols