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We introduce stochastic techniques for simulating polaritons resulting fromlarge molecular aggregate crystals ($10^8$ dyes) in realistic cavities. Thisenables the study of 2D polaritons that are derived from systems with internalexcitonic structure and interact with many modes of cavity light due to theirlarge size, achieving thermodynamic convergence in both the molecular andphotonic subsystems. We demonstrate cases where cavity coupling may induceemergent delocalization not present outside of the cavity. Such examplesdemonstrate the nontrivial role the internal aggregate Hamiltonian can play inpolariton properties.

Polaritons in Large Stochastic Simulations of 2D Molecular Aggregates