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The formation and stability of a sulfur-rich surface of the zinc blende ZnS(001) single crystal have been examined by x-ray photoemission spectroscopy(XPS), low-energy electron diffraction (LEED), and density-functional theory(DFT) calculations. LEED patterns obtained from ZnS (001) surface prepared inultrahigh vacuum conditions are compatible to the formation of the ($1 \times2$) reconstruction. Further XPS investigation is consistent with the conversionof the surface region into a sulfur-rich surface. DFT calculations support theS-richer ZnS surface hypothesis and the indirect notion of increasing in theconductivity of such a new structure.

Zinc blende ZnS (001) surface structure investigated by XPS,LEED and DFT