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Quantum coherent control of bimolecular collisions beyond the ultracoldregime can face a major challenge due to the incoherent addition of differentpartial wave contributions to the total scattering cross section. Thesecontributions become increasingly numerous as the collision energy increases,leading to a loss of overall control. Here, we overcome this limitation byleveraging the recently discovered Partial Wave Phase Locking (PWPL) effect,which synchronizes the oscillations of all partial wave contributions. By usingrigorous quantum scattering calculations, we demonstrate that PWPL enablescoherent control of spin exchange in ion-atom collisions, far outside theultracold regime, even with as many as 5000 partial wave contributions. Thepredicted extent of control is sufficient to be measurable in cold atom-ionhybrid experiments.

Robust Coherent Control of Bimolecular Collisions beyond the Ultracold Regime