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With the development of high-speed electron detectors, four-dimensionalscanning transmission electron microscopy (4D-STEM) has emerged as a powerfultool for characterizing microstructures in material science and life science.However, the complexity of 4D-STEM data processing necessitates an intuitivegraphical user interface software for researchers. In this regard, we havedeveloped 4D-Explorer, an open-source, lightweight and extensible software forprocessing 4D-STEM data. It offers a visual and interactive workflow, includingdata preparation, calibration, image reconstruction and generating quantitativeresults. Furthermore, during calibration, our software includes a novelalgorithm for rotational offset correction that uses a defocused 4D-STEMdataset and its axial bright field image, which has lower experimentalrequirements than conventional methods. We anticipate that 4D-Explorer willhelp researchers harness the capabilities of 4D-STEM technology.

4D-Explorer: A visual software for 4D-STEM data processing and image reconstruction