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Multiferroic particulate composites $(1-x)$Ba$_{0.95}$Ca$_{0.05}$Ti$_{0.89}$Sn$_{0.11}$O$_3$-$(x)$CoFe$_2$O$_4$ with ($x$= 0.1, 0.2, 0.3, 0.4 and 0.5) have been prepared by mechanical mixing of thecalcined and milled individual ferroic phases. X-ray diffraction and Ramanspectroscopy analysis confirmed the formation of both perovskiteBa$_{0.95}$Ca$_{0.05}$Ti$_{0.89}$Sn$_{0.11}$O$_3$ (BCTSn) and spinelCoFe$_2$O$_4$ (CFO) phases without the presence of additional phases. Themorphological properties of the composites were provided by using FieldEmission Scanning Electron Microscopy. The BCTSn-CFO composites exhibitmultiferroic behavior at room temperature, as evidenced by ferroelectric andferromagnetic hysteresis loops. The magnetoelectric (ME) coupling was measuredunder a magnetic field up to 10 kOe and the maximum ME response found to be 0.1mV /cm/ Oe for the composition 0.7 BCTSn-0.3 CFO exhibiting a high degree ofpseudo-cubicity and large density.

Room-temperature magnetoelectric effect in lead-free multiferroic  $(1-x)$ Ba$_{0.95}$Ca$_{0.05}$Ti$_{0.89}$Sn$_{0.11}$O$_3$-$(x)$CoFe$_2$O$_4$  particulate composites