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Nanoscale molecular junctions are celebrated nanoelectronic devices formimicking several electronic functions including rectifiers, sensors, wires,switches, transistors, and memory but capacitive behavior is nearly unexplored.Capacitors are crucial energy storage devices that store energy in the form ofelectrical charges. A capacitor utilizes two electrical conductors separated bya dielectric material. However, many oxides-based dielectrics are well-studiedfor integrating capacitors, however, capacitors comprised of thin-filmmolecular layers are not well-studied. The present work describeselectrochemically grafted thin films of benzimidazole (BENZ) grown on patternedITO electrodes on which a 50 nm Al is deposited to fabricate large-scale (500 x500 micron2) molecular junctions. The nitrogen and sulfur-containing molecularjunctions, ITO/BENZ/Al act as a parallel-plate capacitor with a maximumcapacitance of ~59.6 to 4.79 microFcm-2. The present system can be an excellentplatform for molecular charge storage for future energy applications.

Dipole-moment induced capacitance in nanoscale molecular junctions