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Circular dichroism is a technologically important phenomenon contrasting theabsorption and resultant emission properties between left- and right-handedcircularly polarized light. While the chiral handedness of systems mainlydetermines the mechanism of the circular dichroism in linear optics, thecounterpart in the nonlinear optical regime is nontrivial. Here, in contrast totraditional nonlinear circular dichroism responses from structured surfaces, wereport on an unprecedented bulk-material-induced circular dichroism of secondharmonic generation with a massive g-factor up to 1.8.

High-g-Factor Phase-Matched Circular Dichroism of Second Harmonic Generation in Chiral Polar Liquids